Let $\rho$ be a bipartite state. Its quantum mutual information is defined as $$\newcommand{\tr}{\operatorname{tr}}I(\rho) = S(\tr_B(\rho)) + S(\tr_A(\rho)) - S(\rho),$$ where $S(\sigma)$ is the von Neumann entropy of $\sigma$. If $\rho$ is pure, then it's easy to see that $I(\rho)=2S(\tr_A(\rho))$. If $\rho$ is also maximally entangled, then $I(\rho) = 2\log d$, with $d$ the dimension of the underlying space. This can also be written as $I(\rho)=2$, taking base-$d$ logarithms.
Now, let $\mu^A,\mu^B$ be some measurements for the first and second party. These will correspond to a joint probability distribution $p(a,b;\rho)\equiv \langle\mu^A_a\otimes\mu^B_b,\rho\rangle$. Let $p,p^A,p^B$ denote the corresponding probability distribution, and its two marginals, respectively. If $X,Y$ denote the random variables describing the corresponding outcomes, we can define a classical mutual information as $$I_{\mu}(\rho) \equiv I(X:Y)\equiv H(p^A) + H(p^B) - H(p),$$ with $H(p)$ the (classical) Shannon entropy of the probability distribution $p$. Note that the maximum value of the classical mutual information, obtained for fully correlated variables, is $\log d$ (without the factor of $2$).
When $I(\rho)=2\log d$, and thus $\rho$ is maximally entangled, the parties can observe correlations in infinitely many (projective) measurement bases: for any choice of measurement basis for $A$, there is a choice of measurement basis for $B$ which gives fully correlated outcomes. On the other hand, $I(\rho)=\log d$ can be obtained with the fully correlated mixed state: $\rho=\frac{1}{d}\sum_i |ii\rangle\!\langle ii|$, but said correlation can only be observed with a fixed choice of basis: unless the parties measure both in the computational basis, their outcomes won't be fully correlated.
Is the above intuition of any value in this context? In other words, can one think of the quantum mutual information being larger than its classical upper bound as being linked to the possibility of observing correlations in multiple measurement bases? Or is it just a red herring?